The couple haven't been seen together in a movie since starring in Mr & Mrs Smith back in 2005, which sparked their real-life love affair, but it is believed they have "an exciting new venture" in the pipeline for the near future.
The 38-year-old actress has reportedly penned the script for the upcoming movie, which will be set in Europe.
Angelina is currently working in post-production on her film Unbroken after she impressed with her directorial debut in The Land of Blood and Honey in 2011.
She also voices the title character in Disney's 'Maleficent', which will hit US cinemas on May 30.
Brad, 50, has just wrapped up filming for the World War II action movie 'Fury', which will hit the big screen in the US on November 14.
Meanwhile, the loved-up duo first went public with their relationship in April 2005, just four months after Brad's divorce from Jennifer Aniston was finalised.
Brad and Angelina went on to get engaged in 2012 and share six children, Maddox, 12, Pax, 10, Zahara, nine, Shiloh, seven, and twins Vivienne and Knox, five, together.
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